Lol, this is fun stuff. The art itself needs some work, but the concept is sound, and even the weird (verging on creepy) looking faces have a lot of charm still, despite the huge eyes.
There is a lot wrong with the color choice, lighting, and (as said before) the unnaturally large eyes that are almost too big to fit in the skull, and it's hard to know where to start, but I guess I'll start with the animation.
As far as the animation goes, it's actually very charming and well done. There's not a lot to say about it as most of the error comes from pixel technique and color choices/usage than the animation or movement of the pixels themselves, so great job on that!
I won't mention the eyes anymore because it's already been established why they're creepy (skull size / huge dilated pupils) but do consider enlarging the skull to suit the eyes better, or at least adding ears and a little more height to the hair on top of the heads if you want to keep the eye detail. Most skulls have the eye sitting at midway from the top of the head, and hair adds more volume to even that, so keep this in mind, as it will be pretty jarring to others to look at without this rule being followed.
The second thing I need to address, but possibly the most important, is color choice.
If you've looked at any of my recent posts in this section, I've mentioned that pixels represent the "reflection" of light and the diffuse scattering (like super-tiny marbles or ball-bearings) bouncing around across the surface of a 3D object. Some hit and others bounce off, and the further away you get from the center-mass of impact, the more scattering (diffuse) bouncing occurs to the point where no light reflects at all (shadow).
Note that shadow is highly contrast to light intensity, so the brighter a color (luminosity), the more contrast you need in the shadow area to offset the intensity for it to look natural.
That being said, you have WAY too little contrast between your light and shadows. Be sure to increase the distance between these shades a LOT more than you have already. You have way too many colors there that contribute next to nothing to the 3D form due to them lacking contrast, and 3D form is key, so without contrast, you cannot have 3D form.
The final thing to consider is that, since you're representing LIGHT and since every light usually has a "color" or tint to it, you should keep in mind that color when picking your colors and remember to tint them heavily depending on how intense that light is against those colors. If you think you've pushed it too far, push it farther just to be sure, but the key is to be sure to pick a hue that is not what you THINK it should be, but instead is what it actually *should* be in relation to the light's color. Also don't forget about shadows -- they have ambient light, and that ambient light has color too. In most cases, it's the color of the sky instead of the light source (i.e. the yellow sun, and the blue sky are your light/shadow colors, respectively, in an outside scene).
That should get you started.
I apologize if I sounded harsh, but hopefully you'll pick up a few useful things from this.